Spina, MassimoBonvin, EricSienkiewicz, AndrzejNáfrádi, BálintForró, LászlóHorváth, Endre2016-02-162016-02-162016-02-162016-01-2510.1038/srep19834https://infoscience.epfl.ch/handle/20.500.14299/123739WOS:000368793600001Spatial positioning of nanocrystal building blocks on a solid surface is a prerequisite for assembling individual nanoparticles into functional devices. Here, we report on the graphoepitaxial liquid-solid growth of nanowires of the photovoltaic compound CH3NH3PbI3 in open nanofluidic channels. The guided growth, visualized in real-time with a simple optical microscope, undergoes through a metastable solvatomorph formation in polar aprotic solvents. The presently discovered crystallization leads to the fabrication of mm2-sized surfaces composed of perovskite nanowires having controlled sizes, cross-sectional shapes, aspect ratios and orientation which have not been achieved thus far by other deposition methods. The automation of this general strategy paves the way towards fabrication of wafer-scale perovskite nanowire thin films well-suited for various optoelectronic devices, e.g. solar cells, lasers, light-emitting diodes and photodetectors.Controlled growth of CH3NH3PbI3 nanowires in arrays of open nanofluidic channelstext::journal::journal article::research article