This Master thesis focus on a preliminary analysis of the experimental data obtained during the PETALE program in the CROCUS reactor at EPFL. The objective of PETALE is to validate neutron nuclear data for stainless steel and its main elements –namely iron, nickel, and chromium– and to contribute to the reduction of their uncertainties. For this purpose, transmission experiments were performed using activation dosimetry in separate reflectors made of the four materials. The manuscript is separated in three main parts. In the first part, after a presentation of the experimental setup, the measured spectra of the irradiated dosimeters are analysed. The results obtained with the methodology developed at EPFL are compared with those obtained by the collaboration partner CEA. The second part details two supplementary studies. First an experiment was performed and analysed to assess the impact of position uncertainties of core centre dosimeters. It was estimated to be 0.14 % for a position uncertainty of ±5 mm. The second study dealt with the estimation of PETALE’s monitors dead time. A dead time correction model was applied on a stable period experiment, and validated against activation dosimetry experiments. The power underestimation was estimated at 5 % at 80 W. The last part presents a comparison between experimental results and Serpent simulations of PETALE’s experiments using the JEFF-3.3 nuclear data library. In total twenty experiments were modelled and compared with their respective experiment. In this preliminary study, the results show a general agreement in the thermal range. An underestimation of the transparency of nickel and chromium for neutron with an energy of 2 MeV is observed. At higher energies, around 8 MeV, the chromium transparency is strongly overestimated. Finally, only a slight overestimation of the transparency to 2 MeV neutron is observed for iron and stainless steel reflectors. Outlooks are provided for the next steps of the analysis and validation, as well as for prospects on a longer term.