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  4. Antiferromagnetic fluctuations and charge carrier localization in ferromagnetic bilayer manganites: electrical resistivity scales exponentially with short-range order controlled by temperature and magnetic field
 
research article

Antiferromagnetic fluctuations and charge carrier localization in ferromagnetic bilayer manganites: electrical resistivity scales exponentially with short-range order controlled by temperature and magnetic field

Perring, T. G.
•
Adroja, D. T.
•
Champion, J. D. M.
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September 2, 2020
Journal of Physics: Condensed Matter

The compound La2-2xSr1+2xMn2O7,x= 0.30-0.40, consists of bilayers of ferromagnetic metallic MnO(2)sheets that are separated by insulating layers. The materials show colossal magnetoresistance-a reduction in resistivity of up to two orders of magnitude in a field of 7 T-at their three-dimensional ordering temperatures,T-C= 90-126 K, and are the layered analogues of the widely studied pseudo-cubic perovskite manganites, R(1-x)A(x)MnO(3)(R = rare earth, A = Ca, Sr, Ba, Pb). Two distinct short-range orderings-antiferromagnetic fluctuations and correlated polarons, which are related to the magnetic and the lattice degrees of freedom respectively-have previously been discovered in La2-2xSr1+2xMn2O7,x= 0.40, and have each been qualitatively connected to the resistivity. Here, in a comprehensive study as a function of both temperature and magnetic field for the different hole-concentrations per Mn site ofx= 0.30 and 0.35, we show that antiferromagnetic fluctuations also appear at temperatures just aboveT(C), and that the intensities of both the antiferromagnetic fluctuations and polaron correlations closely track the resistivity. In particular, forx= 0.35 we show that there is a simple scaling relation between the intensities of the antiferromagnetic fluctuations and the in-plane resistivity that applies for the temperatures and magnetic fields used in the experiments. The results show that antiferromagnetic fluctuations are a common feature of La(2-2x)Sr(1+2x)Mn(2)O(7)with ferromagnetic bilayers, and that there is a close connection between the antiferromagnetic fluctuations and polarons in these materials.

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Type
research article
DOI
10.1088/1361-648X/ab88f1
Web of Science ID

WOS:000546885600001

Author(s)
Perring, T. G.
Adroja, D. T.
Champion, J. D. M.
Aeppli, G.  
Chaboussant, G.
Kimura, T.
Tokura, Y.
Manuel, P.
Date Issued

2020-09-02

Published in
Journal of Physics: Condensed Matter
Volume

32

Issue

37

Article Number

374013

Subjects

Physics, Condensed Matter

•

Physics

•

magnetic phase transitions

•

charge carrier localization

•

short range order

•

2-dimensional anti-ferromagnets

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spin fluctuations

•

giant magnetoresistance

•

transition

Editorial or Peer reviewed

REVIEWED

Written at

EPFL

EPFL units
LTM  
Available on Infoscience
July 23, 2020
Use this identifier to reference this record
https://infoscience.epfl.ch/handle/20.500.14299/170315
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