Set-up for broadband Fourier-transform multidimensional electronic spectroscopy

We present a compact passively phase-stabilized ultra-broadband 2D Fourier transform setup. A gas (argon)-filled hollow core fiber pumped by an amplified Ti:Al2O3 laser is used as a light source providing spectral range spanning from 420 to 900 nm. Sub-10-fs pulses were obtained using a deformable mirror-based pulse shaper. We probe the nonlinear response of Rhodamine 101 using 90 nm bandwidth and resolve vibrational coherences of 150 fs period in the ground state. (C) 2015 Optical Society of America


Published in:
Optics Letters, 40, 3, 312-315
Year:
2015
Publisher:
Washington, Optical Society of America
ISSN:
0146-9592
Laboratories:




 Record created 2015-05-29, last modified 2018-03-17


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