000196902 001__ 196902
000196902 005__ 20181203023431.0
000196902 0247_ $$2doi$$a10.1016/j.elspec.2012.11.009
000196902 022__ $$a0368-2048
000196902 02470 $$2ISI$$a000329376800012
000196902 037__ $$aARTICLE
000196902 245__ $$aBetween photocatalysis and photosynthesis: Synchrotron spectroscopy methods on molecules and materials for solar hydrogen generation
000196902 260__ $$aAmsterdam$$bElsevier$$c2013
000196902 269__ $$a2013
000196902 300__ $$a13
000196902 336__ $$aJournal Articles
000196902 520__ $$aEnergy research is to a large extent materials research, encompassing the physics and chemistry of materials, including their synthesis, processing toward components and design toward architectures, allowing for their functionality as energy devices, extending toward their operation parameters and environment, including also their degradation, limited life, ultimate failure and potential recycling. In all these stages, X-ray and electron spectroscopy are helpful methods for analysis, characterization and diagnostics for the engineer and for the researcher working in basic science.This paper gives a short overview of experiments with X-ray and electron spectroscopy for solar energy and water splitting materials and addresses also the issue of solar fuel, a relatively new topic in energy research. The featured systems are iron oxide and tungsten oxide as photoanodes, and hydrogenases as molecular systems. We present surface and subsurface studies with ambient pressure XPS and hard X-ray XPS, resonant photoemission, light induced effects in resonant photoemission experiments and a photo-electrochemical in situ/operando NEXAFS experiment in a liquid cell, and nuclear resonant vibrational spectroscopy (NRVS). (C) 2012 Elsevier B.V. All rights reserved.
000196902 6531_ $$aXAFS
000196902 6531_ $$aVB-PES
000196902 6531_ $$aPhotoelectrochemistry
000196902 6531_ $$aArtificial photosynthesis
000196902 6531_ $$aValence band
000196902 6531_ $$aHole doping
000196902 6531_ $$aCharge transfer
000196902 6531_ $$aSolar fuels
000196902 6531_ $$aSolar hydrogen
000196902 6531_ $$aPhotocatalysis
000196902 6531_ $$aResonant photoemission
000196902 6531_ $$aPhoto-electrochemistry
000196902 6531_ $$aX-ray absorption
000196902 6531_ $$aRIXS
000196902 6531_ $$aHAX-PES
000196902 6531_ $$aAP-XPS
000196902 6531_ $$aNRVS
000196902 6531_ $$aSurface defects
000196902 6531_ $$aBulk defects
000196902 6531_ $$aHydrogenase
000196902 6531_ $$aHematite
000196902 6531_ $$aTungsten oxide
000196902 6531_ $$aWater splitting
000196902 700__ $$aBora, Debajeet K.$$uEmpa, Swiss Fed Labs Mat Sci & Technol, Lab High Performance Ceram, CH-8600 Dubendorf, Switzerland
000196902 700__ $$aHu, Yelin$$uUniv Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA
000196902 700__ $$aThiess, Sebastian$$uDeutsch Elektronen Synchrotron DESY, D-22603 Hamburg, Germany
000196902 700__ $$aErat, Selma$$uEmpa, Swiss Fed Labs Mat Sci & Technol, Lab High Performance Ceram, CH-8600 Dubendorf, Switzerland
000196902 700__ $$aFeng, Xuefei$$uUniv Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA
000196902 700__ $$aMukherjee, Sumanta$$uIndian Inst Sci, Solid State & Struct Chem Unit, Bangalore 560012, Karnataka, India
000196902 700__ $$aFortunato, Giuseppino$$uEmpa, Swiss Fed Labs Mat Sci & Technol, Lab Adv Fibers, CH-9014 St Gallen, Switzerland
000196902 700__ $$aGaillard, Nicolas$$uUniv Hawaii Manoa, Hawaii Nat Energy Inst, Honolulu, HI 96822 USA
000196902 700__ $$aToth, Rita$$uEmpa, Swiss Fed Labs Mat Sci & Technol, Lab High Performance Ceram, CH-8600 Dubendorf, Switzerland
000196902 700__ $$aGajda-Schrantz, Krisztina$$uEmpa, Swiss Fed Labs Mat Sci & Technol, Lab High Performance Ceram, CH-8600 Dubendorf, Switzerland
000196902 700__ $$aDrube, Wolfgang$$uDeutsch Elektronen Synchrotron DESY, D-22603 Hamburg, Germany
000196902 700__ $$0240191$$aGraetzel, Michael$$g105292$$uEcole Polytech Fed Lausanne, Lab Photon & Interfaces, CH-1005 Lausanne, Switzerland
000196902 700__ $$aGuo, Jinghua$$uUniv Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA
000196902 700__ $$aZhu, Junfa$$uUniv Sci & Technol China, Natl Synchrotron Radiat Lab, Hefei 230029, Peoples R China
000196902 700__ $$aConstable, Edwin C.$$uUniv Basel, Dept Chem, CH-4052 Basel, Switzerland
000196902 700__ $$aSarma, D. D.$$uIndian Inst Sci, Solid State & Struct Chem Unit, Bangalore 560012, Karnataka, India
000196902 700__ $$aWang, Hongxin$$uUniv Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA
000196902 700__ $$aBraun, Artur$$uEmpa, Swiss Fed Labs Mat Sci & Technol, Lab High Performance Ceram, CH-8600 Dubendorf, Switzerland
000196902 773__ $$j190$$q93-105$$tJournal Of Electron Spectroscopy And Related Phenomena
000196902 909C0 $$0252060$$pLPI$$xU10101
000196902 909CO $$ooai:infoscience.tind.io:196902$$pSB$$particle
000196902 917Z8 $$x105528
000196902 937__ $$aEPFL-ARTICLE-196902
000196902 973__ $$aEPFL$$rREVIEWED$$sPUBLISHED
000196902 980__ $$aARTICLE