On the interplay between charge, spin and structural dynamics in transition metal complexes

This perspective presents some recent results concerning ultrafast intramolecular relaxation processes in metal-based molecular complexes. Ultrafast electronic/vibrational relaxation at sub-vibrational time scales, ultrafast intersystem crossing processes and ultrafast structure changes are discussed, stressing the questions that still need to be solved in order to arrive at a rationale that describes these processes. We will also discuss some new techniques, based on core-level spectroscopies that can provide new insights into the ultrafast intramolecular relaxation in these systems.


Published in:
Dalton Transactions, 41, 42, 13022-13029
Year:
2012
Publisher:
Cambridge, Royal Soc Chemistry
ISSN:
1477-9226
Laboratories:




 Record created 2013-02-27, last modified 2018-03-17


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