000183804 001__ 183804
000183804 005__ 20181203022945.0
000183804 0247_ $$2doi$$a10.1016/j.chemosphere.2012.11.002
000183804 02470 $$2ISI$$a000315248200016
000183804 037__ $$aARTICLE
000183804 245__ $$aA high-resolution historical record of nutrients, trace elements and organochlorines (DDT and PCB) deposition in a drinking water reservoir (Lake Brêt, Switzerland) points at local and regional pollutant sources
000183804 269__ $$a2013
000183804 260__ $$aOxford$$bPergamon-Elsevier Science Ltd$$c2013
000183804 300__ $$a9
000183804 336__ $$aJournal Articles
000183804 520__ $$aThe 137Cs and 210Pb dating of a 61-cm long sediment core retrieved from a drinking water reservoir (Lake Bret) located in Switzerland revealed a linear and relatively high sedimentation rate (∼1 cm/year) over the last decades. The continuous centimeter scale measurements of physical (porewater and granulometry), organic (Corg, P, N, HI and OI index) and mineral (Cmin and lithogenic trace elements) parameters therefore enables reconstructing the environmental history of the lake and anthropogenic pollutant input (trace metals, DDT and PCBs) at high resolution. A major change in the physical properties of the lowermost sediments occured following the artificial rise of the dam in 1922. After ca. 1940, there was a long-term up-core increase in organic matter deposition attributed to enhance primary production and anoxic bottom water conditions, due to excessive nutrient input from a watershed predominantly used for agriculture that also received domestic effluents from two wastewater-treatment plants. This pattern contrasts with the terrigenius element input (Eu, Sc, Mg, Ti, Al, and Fe) which doubled after the rising of the dam but continuously decreased during the last 60 years. By comparison, the trace metals (Cu, Pb and Hg) present a slight enrichment factor (EF) only during the second part of the 20th century. Although maximum EF Pb (>2) occurred synchronously with the use of leaded gasoline in Switzerland (between ca. 1947 and 1985) the Hg and Cu profiles exhibited a relatively similar trend than Pb during the 20th century, therefore excluding the alkyl-lead added to petrol as the dominant (atmospheric) source of lead input to Lake Brêt. Conversely, the Cu profile that did not follow the decrease registered in Pb and Hg, suggesting an additional source of Cu probably linked to the impact of agricultural activities in the area. In absence of heavy industries in the catchment, the atmospheric deposition of DDT and PCBs via surface runoff follows the historical emissions of POPs in Switzerland. Such result highlights the regional contamination of freshwater resources by the large-scale emission of toxic industrial chemicals in the 1960s and 1970s as well as the efficiency of the regulatory measures subsequently taken.
000183804 6531_ $$asediments
000183804 6531_ $$adrinking water reservoir
000183804 6531_ $$atrace elements
000183804 6531_ $$aorganochlorines
000183804 6531_ $$aorganic matter
000183804 700__ $$aThevenon, Florian
000183804 700__ $$0240229$$ade Alencastro, Luiz$$g104872
000183804 700__ $$0241380$$aLoizeau, Jean-Luc$$g105298
000183804 700__ $$aAdatte, Thierry
000183804 700__ $$0241380$$aGrandjean, Dominique$$g105298
000183804 700__ $$aWildi, Walter
000183804 700__ $$aPoté, John
000183804 773__ $$j90$$q2444–2452$$tChemosphere
000183804 909C0 $$0252083$$pGR-CEL$$xU11838
000183804 909CO $$ooai:infoscience.tind.io:183804$$particle$$pENAC
000183804 917Z8 $$x104872
000183804 937__ $$aEPFL-ARTICLE-183804
000183804 973__ $$aOTHER$$rREVIEWED$$sPUBLISHED
000183804 980__ $$aARTICLE