Ground State of the Quasi-1D Compound BaVS3 Resolved by Resonant Magnetic X-Ray Scattering

Resonant magnetic x-ray scattering near the vanadium L-2,L-3-absorption edges has been used to investigate the low temperature magnetic structure of high quality BaVS3 single crystals. Below T-N = 31 K, the strong resonance revealed a triple-incommensurate magnetic ordering at the wave vector (0.226 0.226 xi) in hexagonal notation, with xi = 0.033. The azimuthal-angle dependence of the scattering signal and time-dependent density functional theory simulations indicate an antiferromagnetic order within the ab plane with the spins polarized along a in the monoclinic structure.


Published in:
Physical Review Letters, 106, -
Year:
2011
Keywords:
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 Record created 2011-12-16, last modified 2018-03-17


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