Direct angle resolved photoemission spectroscopy and superconductivity of strained high-T-c films
Since 1997 we systematically perform direct angle resolved photoemission spectroscopy (ARPES) on in-situ grown thin (<30 nm) cuprate films. Specifically, we probe low-energy electronic structure and properties of high-T-c superconductors (HTSC) under different degrees of epitaxial (compressive vs. tensile) strain. In overdoped and underdoped in-plane compressed (the strain is induced by the choice of substrate) 15 nm thin La2-xSrxCuO4 (LSCO) films we almost double T-c to 40 K, from 20 K and 24 K, respectively. Yet the Fermi surface (FS) remains essentially two-dimensional. In contrast, ARPES data under tensile strain exhibit the dispersion that is three-dimensional, yet T-c drastically decreases. It seems that the in-plane compressive strain tends to push the apical oxygen far away from the CuO2 plane, enhances the two-dimensional character of the dispersion and increases T-c, while the tensile strain acts in the opposite direction and the resulting dispersion is three-dimensional. We have established the shape of the FS for both cases, and all our data are consistent with other ongoing studies, like EXAFS. As the actual lattice of cuprates is like a 'Napoleon-cake', i.e. rigid CuO2 planes alternating with softer 'reservoir', that distort differently under strain, our data rule out all oversimplified two-dimensional (rigid lattice) mean field models. The work is still in progress on optimized La,doped Bi-2201 films with enhanced T-c.
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Keywords: condensed matter physics ; high-T-c superconductivity ; electronic properties ; photoemission spectroscopy ; angle resolved photoemission spectroscopy ; cuprates ; films ; strain ; pulsed laser deposition ; High-Temperature Superconductors ; Thin-Films
Record created on 2010-11-30, modified on 2016-08-09