Repository logo

Infoscience

  • English
  • French
Log In
Logo EPFL, École polytechnique fédérale de Lausanne

Infoscience

  • English
  • French
Log In
  1. Home
  2. Academic and Research Output
  3. Journal articles
  4. State-to-state studies of intramolecular dynamics and unimolecular reactions
 
research article

State-to-state studies of intramolecular dynamics and unimolecular reactions

Kuhn, B
•
Boyarkin, OV  
•
Rizzo, TR  
1997
BERICHTE DER BUNSEN-GESELLSCHAFT

Double-resonance vibrational overtone excitation spectra of small molecules, in combination with laser-induced fluorescence product detection, provide information on both their energetics and intramolecular energy redistribution dynamics. Application of this approach to measure OH stretch overtone spectra of HOOH and NH2OH near their dissociation threshold provides estimates of the O-O and N-O bond energies of 17051.8 +/- 4 cm(-1) and 21 620 +/- 20 cm(-1) respectively. In symmetrical molecules, such as HOOH, the double-resonance excitation technique allows us to prepare molecules in either pure OH stretch overtone levels or combination levels in which the excitation energy is divided between two identical OH stretch oscillators. Comparison of the resulting vibrational overtone linewidths indicates no clear difference between the pure OH stretch and the local-local combination levels. However, comparison of the energy transfer rates from pure OH stretch vibrations and those in which one quantum of energy is put in a low frequency mode reveals faster rates from the latter. This observation clearly indicates that coupling strengths depend markedly on the vibrational character of the coupling partner and not simply on the total energy. Comparison of the OH stretch overtone spectra of the structurally similar molecules HOOH, NH2OH, and CH3OH reveal similar rates of vibrational energy redistribution, despite the difference in the density of states in these molecules. This observation reinforces the notion that energy flow between the OH stretch and dark background states is not statistical but rather is controlled by coupling to a small subset of background states.

  • Details
  • Metrics
Type
research article
DOI
10.1002/bbpc.19971010305
Author(s)
Kuhn, B
Boyarkin, OV  
Rizzo, TR  
Date Issued

1997

Published in
BERICHTE DER BUNSEN-GESELLSCHAFT
Volume

101

Issue

3

Start page

339

End page

345

Editorial or Peer reviewed

REVIEWED

Written at

EPFL

EPFL units
LCPM  
Available on Infoscience
December 15, 2005
Use this identifier to reference this record
https://infoscience.epfl.ch/handle/20.500.14299/221329
Logo EPFL, École polytechnique fédérale de Lausanne
  • Contact
  • infoscience@epfl.ch

  • Follow us on Facebook
  • Follow us on Instagram
  • Follow us on LinkedIn
  • Follow us on X
  • Follow us on Youtube
AccessibilityLegal noticePrivacy policyCookie settingsEnd User AgreementGet helpFeedback

Infoscience is a service managed and provided by the Library and IT Services of EPFL. © EPFL, tous droits réservés