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conference paper

Observing spectral fluctuations in single nanocrystals across multiple time scales

Conradt, Frieder
•
Gebauer, Philipp
•
Zhu, Chenglian
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Herink, Georg
•
Solli, Daniel R.
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March 19, 2025
Real-time Measurements, Rogue Phenomena, and Single-Shot Applications X
Real-time Measurements, Rogue Phenomena, and Single-Shot Applications X

While at cryogenic temperatures, quantum dots generate single photons at a narrowband spectrum, temporal fluctuations in its peak position pose a significant challenge towards control and metrology protocols. Up to date, evidences of spectral fluctuations are by large measured indirectly. In this work, heralded spectroscopy is used to directly measure spectral fluctuations for single CsPbBr3 nanocrystals across 8 orders of magnitude in time, down to the microsecond. We find that spectral noise spans this entire temporal range with a weak power-law dependence and critically enhance with the excitation power, demonstrating a clear tradeoff between brightness and spectral stability. Further systematic studies of the parameters that determine the amplitude and time scale of spectral diffusion will aim to clarify its underlying mechanism with the outlook of synthetically overcoming this challenge.

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Type
conference paper
DOI
10.1117/12.3049971
Author(s)
Conradt, Frieder

University of Konstanz

Gebauer, Philipp

University of Konstanz

Zhu, Chenglian

ETH Zurich

Haage, Eva

University of Konstanz

Cherniukh, Ihor

ETH Zurich

Bruschini, Claudio  

EPFL

Rainò, Gabriele

ETH Zurich

Charbon, Edoardo  

EPFL

Kovalenko, Maksym V.

ETH Zurich

Leitenstorfer, Alfred

University of Konstanz

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Editors
Herink, Georg
•
Solli, Daniel R.
•
Bielawski, Serge
Date Issued

2025-03-19

Publisher

SPIE

Published in
Real-time Measurements, Rogue Phenomena, and Single-Shot Applications X
Series title/Series vol.

Proceedings SPIE; PC13348

Start page

17

Editorial or Peer reviewed

REVIEWED

Written at

EPFL

EPFL units
AQUA  
Event nameEvent acronymEvent placeEvent date
Real-time Measurements, Rogue Phenomena, and Single-Shot Applications X

LASE

San Francisco, United States

2025-01-25 - 2025-01-31

Available on Infoscience
December 24, 2025
Use this identifier to reference this record
https://infoscience.epfl.ch/handle/20.500.14299/257309
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