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research article

Non-Kolmogorov-Avrami switching kinetics in ferroelectric thin films

Tagantsev, A. K.  
•
Stolichnov, I.  
•
Setter, N.  
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2002
Physical Review B

The switching kinetics in ferroelectric thin films has been intensively studied during the past decade. It is widely accepted that this kinetics is basically governed by the dynamics of domain coalescence (the Kolmogorov-Avrami-Ishibashi model). This conclusion is mainly supported by fitting the time dependence of the switching currents to that predicted by this model, the fit being typically performed in a 1-2 decade interval of time. The present paper reports on a study of the switching kinetics in modified Pt/Pb(Zr,Ti)O-3/Pt thin films as a function of time and applied voltage, performed in time intervals from 10 ns to 1s. Our experimental data show that both the time and applied field dependences of the switching polarization (when monitored over a wide enough time interval) are in a strong qualitative disagreement with the predictions of the Kolmogorov-Avrami-Ishibashi approach. For the interpretation of our result, an alternative approach is forwarded. In contrast to Kolmogorov-Avrami-Ishibashi approach, we assume that the film consists of many areas, which have independent switching dynamics. The switching in an area is considered to be triggered by an act of the reverse domain nucleation. The switching kinetics is described in terms of the distribution function of the nucleation probabilities in these areas. The developed approach enables a good description of the polarization dynamics in typical ferroelectric thin films for memory applications.

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Type
research article
DOI
10.1103/PhysRevB.66.214109
Web of Science ID

WOS:000180318800038

Author(s)
Tagantsev, A. K.  
Stolichnov, I.  
Setter, N.  
Cross, J. S.
Tsukada, M.
Date Issued

2002

Published in
Physical Review B
Volume

66

Issue

21

Article Number

214109

Subjects

switchable polarization fatigue

•

e hysteresis loop

•

suppression

•

capacitors

•

electrodes

•

scenarios

•

model

Note

Tagantsev, AK Ecole Polytech Fed Lausanne, Ceram Lab, CH-1015 Lausanne, Switzerland Ecole Polytech Fed Lausanne, Ceram Lab, CH-1015 Lausanne, Switzerland Fujitsu Labs Ltd, Atsugi, Kanagawa 2430197, Japan

634AX

Cited References Count:25

Editorial or Peer reviewed

REVIEWED

Written at

EPFL

EPFL units
LC  
Available on Infoscience
August 21, 2006
Use this identifier to reference this record
https://infoscience.epfl.ch/handle/20.500.14299/233495
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