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research article
Ultrafast Structural Dynamics along the beta - gamma Phase Transition Path in MnAs
April 9, 2019
We investigate the orthorhombic distortion and the structural dynamics of epitaxial MnAs layers on GaAs(001) using static and time-resolved x-ray diffraction. Laser-induced intensity oscillations of Bragg reflections allow us to identify the optical phonon associated with orthorhombic distortion and to follow its softening along the path towards an undistorted phase of hexagonal symmetry. The frequency of this mode falls in the THz range, in agreement with recent calculations. Incomplete softening suggests that the beta - gamma transformation deviates from a purely second-order displacive transition.
Type
research article
Web of Science ID
WOS:000463902800013
Authors
Vidal, Franck
•
Zheng, Yunlin
•
Lounis, Lounes
•
Coelho, Leticia
•
Laulhe, Claire
•
Spezzani, Carlo
•
Ciavardini, Alessandra
•
Popescu, Horia
•
•
Allaria, Enrico
Publication date
2019-04-09
Publisher
Published in
Volume
122
Issue
14
Article Number
145702
Peer reviewed
REVIEWED
EPFL units
Available on Infoscience
June 18, 2019
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