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research article

Tunable Carrier Multiplication and Cooling in Graphene

Johannsen, Jens Christian  
•
Ulstrup, Soren
•
Crepaldi, Alberto  
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2015
Nano Letters

Time- and angle-resolved photoemission measurements on two doped graphene samples displaying different doping levels reveal remarkable differences in the ultrafast dynamics of the hot carriers in the Dirac cone. In the more strongly (n-)doped graphene, we observe larger carrier multiplication factors (>3) and a significantly faster phonon-mediated cooling of the carriers back to equilibrium compared to in the less (p-)doped graphene. These results suggest that a careful tuning of the doping level allows for an effective manipulation of graphene's dynamical response to a photoexcitation. © 2014 American Chemical Society.

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Type
research article
DOI
10.1021/nl503614v
Web of Science ID

WOS:000348086100052

Author(s)
Johannsen, Jens Christian  
Ulstrup, Soren
Crepaldi, Alberto  
Cilento, Federico
Zacchigna, Michele
Miwa, Jill A.
Cacho, Cephise
Chapman, Richard T.
Springate, Emma
Fromm, Felix
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Date Issued

2015

Publisher

Amer Chemical Soc

Published in
Nano Letters
Volume

15

Issue

1

Start page

326

End page

331

Subjects

carrier multiplication

•

charge carrier tunability

•

epitaxial graphene

•

hot carrier dynamics

•

time-resolved ARPES

Editorial or Peer reviewed

REVIEWED

Written at

EPFL

EPFL units
LSE  
Available on Infoscience
May 29, 2015
Use this identifier to reference this record
https://infoscience.epfl.ch/handle/20.500.14299/114517
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