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research article

2022 roadmap on low temperature electrochemical CO2 reduction

Stephens, Ifan E. L.
•
Chan, Karen
•
Bagger, Alexander
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October 1, 2022
Journal Of Physics-Energy

Electrochemical CO2 reduction (CO2R) is an attractive option for storing renewable electricity and for the sustainable production of valuable chemicals and fuels. In this roadmap, we review recent progress in fundamental understanding, catalyst development, and in engineering and scale-up. We discuss the outstanding challenges towards commercialization of electrochemical CO2R technology: energy efficiencies, selectivities, low current densities, and stability. We highlight the opportunities in establishing rigorous standards for benchmarking performance, advances in in operando characterization, the discovery of new materials towards high value products, the investigation of phenomena across multiple-length scales and the application of data science towards doing so. We hope that this collective perspective sparks new research activities that ultimately bring us a step closer towards establishing a low- or zero-emission carbon cycle.

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Type
research article
DOI
10.1088/2515-7655/ac7823
Web of Science ID

WOS:000863502400001

Author(s)
Stephens, Ifan E. L.
Chan, Karen
Bagger, Alexander
Boettcher, Shannon W.
Bonin, Julien
Boutin, Etienne  
Buckley, Aya K.
Buonsanti, Raffaella  
Cave, Etosha R.
Chang, Xiaoxia
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Date Issued

2022-10-01

Publisher

IOP Publishing Ltd

Published in
Journal Of Physics-Energy
Volume

4

Issue

4

Article Number

042003

Subjects

Energy & Fuels

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Materials Science, Multidisciplinary

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Energy & Fuels

•

Materials Science

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electrocatalysis

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co2 reduction

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electrochemistry

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solar fuels

•

carbon-dioxide capture

•

electrocatalytic conversion

•

selective electroreduction

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technoeconomic analysis

•

accelerated discovery

•

mechanistic insights

•

bipolar membranes

•

metal-electrodes

•

structural basis

•

liquid fuel

Editorial or Peer reviewed

REVIEWED

Written at

EPFL

Available on Infoscience
October 24, 2022
Use this identifier to reference this record
https://infoscience.epfl.ch/handle/20.500.14299/191649
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