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  4. Three-Dimensional Electron Realm in VSe2 by Soft-X-Ray Photoelectron Spectroscopy: Origin of Charge-Density Waves
 
research article

Three-Dimensional Electron Realm in VSe2 by Soft-X-Ray Photoelectron Spectroscopy: Origin of Charge-Density Waves

Strocov, Vladimir N.
•
Shi, Ming
•
Kobayashi, Masaki
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2012
Physical Review Letters

The resolution of angle-resolved photoelectron spectroscopy (ARPES) in three-dimensional (3D) momentum k is fundamentally limited by ill defined surface-perpendicular wave vector k(perpendicular to) associated with the finite photoelectron mean free path. Pushing ARPES into the soft-x-ray energy region sharpens the k(perpendicular to) definition, allowing accurate electronic structure investigations in 3D materials. We apply soft-x-ray ARPES to explore the 3D electron realm in a paradigm transition metal dichalcogenide VSe2. Essential to break through the dramatic loss of the valence band photoexcitation cross section at soft-x-ray energies is the advanced photon flux performance of our synchrotron instrumentation. By virtue of the sharp 3D momentum definition, the soft-x-ray ARPES experimental band structure and Fermi surface of VSe2 show a textbook clarity. We identify pronounced 3D warping of the Fermi surface and show that its concomitant nesting acts as the precursor for the exotic 3D charge-density waves in VSe2. Our results demonstrate the immense potential of soft-x-ray ARPES to explore details of 3D electronic structure.

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Type
research article
DOI
10.1103/PhysRevLett.109.086401
Web of Science ID

WOS:000307711300014

Author(s)
Strocov, Vladimir N.
Shi, Ming
Kobayashi, Masaki
Monney, Claude
Wang, Xiaoqiang  
Krempasky, Juraj
Schmitt, Thorsten
Patthey, Luc
Berger, Helmuth  
Blaha, Peter
Date Issued

2012

Publisher

Amer Physical Soc

Published in
Physical Review Letters
Volume

109

Issue

8

Article Number

086401

Editorial or Peer reviewed

REVIEWED

Written at

EPFL

EPFL units
LSE  
Available on Infoscience
February 27, 2013
Use this identifier to reference this record
https://infoscience.epfl.ch/handle/20.500.14299/89658
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