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research article

Inhomogeneity of charge-density-wave order and quenched disorder in a high-T-c superconductor

Campi, G.
•
Bianconi, A.
•
Poccia, N.
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2015
Nature

It has recently been established that the high-transition-temperature (high-T-c) superconducting state coexists with short-range charge-density-wave order(1-11) and quenched disorder(12,13) arising from dopants and strain(14-17). This complex, multiscale phase separation(18-21) invites the development of theories of high-temperature superconductivity that include complexity(22-25). The nature of the spatial interplay between charge and dopant order that provides a basis for nanoscale phase separation remains a key open question, because experiments have yet to probe the unknown spatial distribution at both the nanoscale and mesoscale (between atomic and macroscopic scale). Here we report micro X-ray diffraction imaging of the spatial distribution of both short-range charge-density-wave 'puddles' (domains with only a few wavelengths) and quenched disorder in HgBa2CuO4+y, the single-layer cuprate with the highest T-c, 95 kelvin (refs 26-28). We found that the charge-density-wave puddles, like the steam bubbles in boiling water, have a fat-tailed size distribution that is typical of self-organization near a critical point(19). However, the quenched disorder, which arises from oxygen interstitials, has a distribution that is contrary to the usually assumed random, uncorrelated distribution(12,13). The interstitial-oxygen-rich domains are spatially anticorrelated with the charge-density-wave domains, because higher doping does not favour the stripy charge-density-wave puddles, leading to a complex emergent geometry of the spatial landscape for superconductivity.

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Type
research article
DOI
10.1038/nature14987
Web of Science ID

WOS:000361297900039

Author(s)
Campi, G.
Bianconi, A.
Poccia, N.
Bianconi, G.
Barba, L.
Arrighetti, G.
Innocenti, D.  
Karpinski, J.
Zhigadlo, N. D.
Kazakov, S. M.
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Date Issued

2015

Publisher

Nature Publishing Group

Published in
Nature
Volume

525

Issue

7569

Start page

359

End page

362

Editorial or Peer reviewed

REVIEWED

Written at

EPFL

EPFL units
LPMC  
Available on Infoscience
December 2, 2015
Use this identifier to reference this record
https://infoscience.epfl.ch/handle/20.500.14299/121233
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