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research article

Tuning Conductivity and Spin Dynamics in Few-Layer Graphene via In Situ Potassium Exposure

Markus, Bence Gabor
•
Sagi, Oliver
•
Kollarics, Sandor
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September 30, 2020
Physica Status Solidi B-Basic Solid State Physics

Chemical modification such as intercalation or doping of novel materials is of great importance for exploratory material science and applications in various fields of physics and chemistry. Herein, the systematic intercalation of chemically exfoliated few-layer graphene with potassium is reported while monitoring the sample resistance using microwave conductivity. It is found that the conductivity of the samples increases by about an order of magnitude upon potassium exposure. The increased number of charge carriers deduced from the electron spin resonance (ESR) intensity also reflects this increment. The doped phases exhibit two asymmetric Dysonian lines in ESR, a usual sign of the presence of mobile charge carriers. The width of the broader component increases with the doping steps; however, the narrow components seem to have a constant line width.

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Type
research article
DOI
10.1002/pssb.202000368
Web of Science ID

WOS:000573689700001

Author(s)
Markus, Bence Gabor
•
Sagi, Oliver
•
Kollarics, Sandor
•
Edelthalhammer, Konstantin F.
•
Hirsch, Andreas
•
Hauke, Frank
•
Szirmai, Peter  
•
Nafradi, Balint  
•
Forro, Laszlo  
•
Simon, Ferenc  
Date Issued

2020-09-30

Published in
Physica Status Solidi B-Basic Solid State Physics
Article Number

2000368

Subjects

Physics, Condensed Matter

•

Physics

•

charge transfer

•

doping

•

electron spin resonance

•

intercalation

•

spintronics

•

cavity perturbation technique

•

graphite lamellar compounds

•

resonance

•

functionalization

•

superconductivity

•

compound

•

metals

•

sodium

•

rbc60

•

c-60

Note

This is an open access article under the terms of the Creative Commons Attribution License.

Peer reviewed

REVIEWED

Written at

EPFL

EPFL units
LPMC  
Available on Infoscience
October 15, 2020
Use this identifier to reference this record
https://infoscience.epfl.ch/handle/20.500.14299/172487
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