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  4. The effect of high relative humidity on a network of water-sensitive particles (couscous) as revealed by in situ X-ray tomography
 
research article

The effect of high relative humidity on a network of water-sensitive particles (couscous) as revealed by in situ X-ray tomography

Vego, Ilija
•
Tengattini, Alessandro
•
Ando, Edward  
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May 30, 2022
Soft Matter

Water significantly influences the mechanical behaviour of all granular materials but none as much as hygroscopic amorphous particles. With sufficiently high water content, particles can swell, agglomerate and their mechanical properties can be reduced, having direct effects on the macroscopic response of the material. In the food and pharmaceutical industry this can cause loss of product functionality. Despite their relevance, very little is known about the microscopic processes that induce these phenomena. Previous studies focused on single particle behaviour, the strength of agglomerated particles and the material flowability, leaving unexplored the link connecting the particle behaviour and the bulk response. This experimental study aims to investigate this aspect with quantitative measurements at both particle and macroscopic scales. A sample of fine couscous is exposed to a high relative humidity (RH) air flow, while being subjected to oedometric conditions, in order to reproduce the storage-silo conditions. In the meantime, X-ray tomographies are acquired continuously and the resulting images are analysed. The designed spatial resolution allows each particle of the sample to be identified and tracked, allowing volumetric evolution to be compared to the properties of the whole sample. The analysis reveals a dilation-compaction macroscopic behaviour, a result of the competition between the particle swelling and the higher deformability as the water content increases. The number, orientations and inter-particle contacts are computed. Their area is related to the applied boundary conditions, and is found to be consistent with the particle swelling and dependent on the applied stress direction.

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Type
research article
DOI
10.1039/d2sm00322h
Web of Science ID

WOS:000811019200001

Author(s)
Vego, Ilija
Tengattini, Alessandro
Ando, Edward  
Lenoir, Nicolas
Viggiani, Gioacchino
Date Issued

2022-05-30

Publisher

ROYAL SOC CHEMISTRY

Published in
Soft Matter
Volume

18

Issue

25

Start page

4747

End page

4755

Subjects

Chemistry, Physical

•

Materials Science, Multidisciplinary

•

Physics, Multidisciplinary

•

Polymer Science

•

Chemistry

•

Materials Science

•

Physics

•

moisture-content

•

physical-properties

•

flowability

•

caking

•

deformation

Editorial or Peer reviewed

REVIEWED

Written at

EPFL

EPFL units
IMAGING  
Available on Infoscience
July 4, 2022
Use this identifier to reference this record
https://infoscience.epfl.ch/handle/20.500.14299/188993
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