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research article

Determining the phase diagram of atomically thin layered antiferromagnet CrCl3

Wang, Zhe
•
Gibertini, Marco  
•
Dumcenco, Dumitru
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December 1, 2019
Nature Nanotechnology

Changes in the spin configuration of atomically thin, magnetic van der Waals multilayers can cause drastic modifications in their opto-electronic properties. Conversely, the opto-electronic response of these systems provides information about the magnetic state, which is very difficult to obtain otherwise. Here, we show that in CrCl3 multilayers, the dependence of the tunnelling conductance on applied magnetic field, temperature and number of layers tracks the evolution of the magnetic state, enabling the magnetic phase diagram to be determined experimentally. Besides a high-field spin-flip transition occurring for all thicknesses, the in-plane magnetoconductance exhibits an even-odd effect due to a low-field spin-flop transition. Through a quantitative analysis of the phenomena, we determine the interlayer exchange coupling as well as the layer magnetization and show that in CrCl3 shape anisotropy dominates. Our results reveal the rich behaviour of atomically thin layered antiferromagnets with weak magnetic anisotropy.

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Type
research article
DOI
10.1038/s41565-019-0565-0
Web of Science ID

WOS:000500925300009

Author(s)
Wang, Zhe
Gibertini, Marco  
Dumcenco, Dumitru
Taniguchi, Takashi
Watanabe, Kenji
Giannini, Enrico
Morpurgo, Alberto F.
Date Issued

2019-12-01

Publisher

Nature Publishing Group

Published in
Nature Nanotechnology
Volume

14

Issue

12

Start page

1116

End page

1122

Subjects

Nanoscience & Nanotechnology

•

Materials Science, Multidisciplinary

•

Science & Technology - Other Topics

•

Materials Science

•

sublattice magnetization

•

spin

•

field

•

ferromagnetism

Editorial or Peer reviewed

REVIEWED

Written at

EPFL

EPFL units
THEOS  
Available on Infoscience
December 19, 2019
Use this identifier to reference this record
https://infoscience.epfl.ch/handle/20.500.14299/164081
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