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research article

Scale-invariant magnetic anisotropy in RuCl(3)at high magnetic fields

Modic, K. A.
•
McDonald, Ross D.
•
Ruff, J. P. C.
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October 5, 2020
Nature Physics

Scale-invariant magnetic anisotropy in RuCl(3)has been revealed through measurements of its magnetotropic coefficient, providing evidence for a high degree of exchange frustration that favours the formation of a spin liquid state. In RuCl3, inelastic neutron scattering and Raman spectroscopy reveal a continuum of non-spin-wave excitations that persists to high temperature, suggesting the presence of a spin liquid state on a honeycomb lattice. In the context of the Kitaev model, finite magnetic fields introduce interactions between the elementary excitations, and thus the effects of high magnetic fields that are comparable to the spin-exchange energy scale must be explored. Here, we report measurements of the magnetotropic coefficient-the thermodynamic coefficient associated with magnetic anisotropy-over a wide range of magnetic fields and temperatures. We find that magnetic field and temperature compete to determine the magnetic response in a way that is independent of the large intrinsic exchange-interaction energy. This emergent scale-invariant magnetic anisotropy provides evidence for a high degree of exchange frustration that favours the formation of a spin liquid state in RuCl3.

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Type
research article
DOI
10.1038/s41567-020-1028-0
Web of Science ID

WOS:000575344700003

Author(s)
Modic, K. A.
McDonald, Ross D.
Ruff, J. P. C.
Bachmann, Maja D.
Lai, You
Palmstrom, Johanna C.
Graf, David
Chan, Mun K.
Balakirev, F. F.
Betts, J. B.
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Date Issued

2020-10-05

Published in
Nature Physics
Volume

17

Start page

240

End page

244

Subjects

Physics, Multidisciplinary

•

Physics

Editorial or Peer reviewed

REVIEWED

Written at

EPFL

EPFL units
QMAT  
Available on Infoscience
October 21, 2020
Use this identifier to reference this record
https://infoscience.epfl.ch/handle/20.500.14299/172648
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