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research article

Microscopic evidence for strong periodic lattice distortion in two-dimensional charge-density wave systems

Dai, Jixia
•
Calleja, Eduardo
•
Alldredge, Jacob
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2014
Physical Review B

In quasi-two-dimensional electron systems of layered transition metal dichalcogenides (TMDs) there is still controversy about the nature of the transitions to charge-density wave (CDW) phases, i.e., whether they are described by a Peierls-type mechanism or by a lattice-driven model. By performing scanning tunneling microscopy experiments on canonical TMD-CDW systems, we image the electronic modulation and the lattice distortion separately in 2H-TaS2, TaSe2, and NbSe2. Across the three materials, we found dominant lattice contributions instead of the electronic modulation expected from Peierls transitions, in contrast to the CDW states, which show the hallmark of contrast inversion between filled and empty states. Our results imply that periodic lattice distortion plays a vital role in the formation of CDW phases in TMDs and illustrate the importance of taking into account the more complicated lattice degrees of freedom when studying correlated electron systems.

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Type
research article
DOI
10.1103/PhysRevB.89.165140
Web of Science ID

WOS:000335797600005

Author(s)
Dai, Jixia
Calleja, Eduardo
Alldredge, Jacob
Zhu, Xiangde
Li, Lijun
Lu, Wenjian
Sun, Yuping
Wolf, Thomas
Berger, Helmuth  
Mcelroy, Kyle
Date Issued

2014

Publisher

Amer Physical Soc

Published in
Physical Review B
Volume

89

Issue

16

Article Number

165140

Editorial or Peer reviewed

REVIEWED

Written at

EPFL

EPFL units
LSE  
Available on Infoscience
June 16, 2014
Use this identifier to reference this record
https://infoscience.epfl.ch/handle/20.500.14299/104330
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