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research article

Carrier Transport Layer-Free Perovskite Solar Cells

Wang, Liang
•
Yang, Shuzhang
•
Han, Qianji
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September 24, 2021
Chemsuschem

Power conversion efficiencies (PCEs) of up to 25.5 % have been reported for perovskite solar cells (PSCs). Thus, they have shown great potential for commercial applications. Therefore, simplifying technological process and reducing production costs have been a widespread concern among scientific and industrial communities. In this study, PSCs are prepared with the simplest device architecture (FTO/MAPbI(3)/carbon). A high-quality perovskite film with few interface defects and good carrier transport is obtained by tuning the p-n properties, matching energy levels, and enhancing carrier collection and transport. A PCE of 12.01 % is achieved, which is the best reported to date for this device structure. The device also shows excellent long-term stability, owing to the elimination of charge transport layers and the usage of hydrophobic materials. This study provides a new approach to reduce production costs and simplify production of PSCs.

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Type
research article
DOI
10.1002/cssc.202101592
Web of Science ID

WOS:000698722000001

Author(s)
Wang, Liang
Yang, Shuzhang
Han, Qianji
Yu, Fengyang
Zhang, Hong  
Cai, Xiaoyong
Zhang, Chu
Gao, Liguo
Ma, Tingli
Date Issued

2021-09-24

Publisher

WILEY-V C H VERLAG GMBH

Published in
Chemsuschem
Volume

14

Issue

21

Start page

4776

End page

4782

Subjects

Chemistry, Multidisciplinary

•

Green & Sustainable Science & Technology

•

Chemistry

•

Science & Technology - Other Topics

•

carbon

•

charge transport

•

perovskites

•

solar cells

•

surface passivation

•

efficiency

•

dynamics

•

contact

Editorial or Peer reviewed

REVIEWED

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EPFL

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Available on Infoscience
October 9, 2021
Use this identifier to reference this record
https://infoscience.epfl.ch/handle/20.500.14299/182056
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