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  4. Proximity-Induced Novel Ferromagnetism Accompanied with Resolute Metallicity in NdNiO3 Heterostructure
 
research article

Proximity-Induced Novel Ferromagnetism Accompanied with Resolute Metallicity in NdNiO3 Heterostructure

Caputo, Marco
•
Ristic, Zoran  
•
Dhaka, Rajendra S.  
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August 11, 2021
Advanced Science

Employing X-ray magnetic circular dichroism (XMCD), angle-resolved photoemission spectroscopy (ARPES), and momentum-resolved density fluctuation (MRDF) theory, the magnetic and electronic properties of ultrathin NdNiO3 (NNO) film in proximity to ferromagnetic (FM) La0.67Sr0.33MnO3 (LSMO) layer are investigated. The experimental data shows the direct magnetic coupling between the nickelate film and the manganite layer which causes an unusual ferromagnetic (FM) phase in NNO. Moreover, it is shown the metal-insulator transition in the NNO layer, identified by an abrupt suppression of ARPES spectral weight near the Fermi level (E-F), is absent. This observation suggests that the insulating AFM ground state is quenched in proximity to the FM layer. Combining the experimental data (XMCD and AREPS) with the momentum-resolved density fluctuation calculation (MRDF) reveals a direct link between the MIT and the magnetic orders in NNO systems. This work demonstrates that the proximity layer order can be broadly used to modify physical properties and enrich the phase diagram of RENiO3 (RE = rare-earth element).

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Type
research article
DOI
10.1002/advs.202101516
Web of Science ID

WOS:000684126100001

Author(s)
Caputo, Marco
Ristic, Zoran  
Dhaka, Rajendra S.  
Das, Tanmoy
Wang, Zhiming
Matt, Christan E.
Plumb, Nicholas C.
Guedes, Eduardo B.
Jandke, Jasmin
Naamneh, Muntaser
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Date Issued

2021-08-11

Published in
Advanced Science
Article Number

2101516

Subjects

Chemistry, Multidisciplinary

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Nanoscience & Nanotechnology

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Materials Science, Multidisciplinary

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Chemistry

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Science & Technology - Other Topics

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Materials Science

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magnetic coupling

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metal-insulator transition

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proximity effect

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metal-insulator-transition

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field

Editorial or Peer reviewed

REVIEWED

Written at

EPFL

EPFL units
LSNS  
Available on Infoscience
August 28, 2021
Use this identifier to reference this record
https://infoscience.epfl.ch/handle/20.500.14299/181023
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