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research article

Nanoscale depth-resolved coherent femtosecond motion in laser-excited bismuth

Johnson, S. L.
•
Beaud, P.
•
Milne, C. J.  
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2008
Physical Review Letters

We employ grazing-incidence femtosecond x-ray diffraction to characterize the coherent, femtosecond laser-induced lattice motion of a bismuth crystal as a function of depth from the surface with a temporal resolution of 193 +/- 8 fs. The data show direct consequences on the lattice motion from carrier diffusion and electron-hole interaction, allowing us to estimate an effective diffusion rate of D=2.3 +/- 0.3 cm(2)/s for the highly excited carriers and an electron-hole interaction time of 260 +/- 20 fs.

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