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research article

Semi-analytical Solutions for Tubular Chemical Reactors

Rodrigues, Diogo  
•
Billeter, Julien  
•
Bonvin, Dominique  
2017
Chemical Engineering Science

The one-dimensional tubular reactor model with advection and possibly axial diffusion is the classical model of distributed chemical reaction systems. This system is described by partial differential equations that depend on the time <i>t</i> and the spatial coordinate <i>z</i>. In this article, semi-analytical solutions to these partial differential equations are developed regardless of the complexity of their initial and boundary conditions and reaction kinetics. These semi-analytical solutions can be used to analyze the effect on the concentrations at the current coordinates <i>z</i> and <i>t</i> of (i) the initial and boundary conditions, and (ii) the reactions that took place at an earlier time. A case study illustrates the application of these results to tubular reactors for the two cases, without and with diffusion.

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Type
research article
DOI
10.1016/j.ces.2017.06.008
Web of Science ID

WOS:000410833900020

Author(s)
Rodrigues, Diogo  
Billeter, Julien  
Bonvin, Dominique  
Date Issued

2017

Publisher

Elsevier

Published in
Chemical Engineering Science
Volume

172

Start page

239

End page

249

Subjects

Partial differential equations

•

Tubular reactors

•

Analytical solutions

•

System decoupling

Editorial or Peer reviewed

REVIEWED

Written at

EPFL

EPFL units
LA  
Available on Infoscience
May 16, 2017
Use this identifier to reference this record
https://infoscience.epfl.ch/handle/20.500.14299/137403
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