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  4. Light-Induced Metastable Hidden Skyrmion Phase in the Mott Insulator Cu2OSeO3
 
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research article

Light-Induced Metastable Hidden Skyrmion Phase in the Mott Insulator Cu2OSeO3

Truc, Benoit  
•
Sapozhnik, Alexey A.
•
Tengdin, Phoebe  
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July 8, 2023
Advanced Materials

The discovery of a novel long-lived metastable skyrmion phase in the multiferroic insulator Cu2OSeO3 visualized with Lorentz transmission electron microscopy for magnetic fields below the equilibrium skyrmion pocket is reported. This phase can be accessed by exciting the sample non-adiabatically with near-infrared femtosecond laser pulses and cannot be reached by any conventional field-cooling protocol, referred as a hidden phase. From the strong wavelength dependence of the photocreation process and via spin-dynamics simulations, the magnetoelastic effect is identified as the most likely photocreation mechanism. This effect results in a transient modification of the magnetic free energy landscape extending the equilibrium skyrmion pocket to lower magnetic fields. The evolution of the photoinduced phase is monitored for over 15 min and no decay is found. Because such a time is much longer than the duration of any transient effect induced by a laser pulse in a material, it is assumed that the newly discovered skyrmion state is stable for practical purposes, thus breaking ground for a novel approach to control magnetic state on demand at ultrafast timescales and drastically reducing heat dissipation relevant for next-generation spintronic devices.

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Type
research article
DOI
10.1002/adma.202304197
Web of Science ID

WOS:001024056200001

Author(s)
Truc, Benoit  
•
Sapozhnik, Alexey A.
•
Tengdin, Phoebe  
•
Bostroem, Emil Vinas
•
Schoenenberger, Thomas
•
Gargiulo, Simone  
•
Madan, Ivan  
•
LaGrange, Thomas  
•
Magrez, Arnaud  
•
Verdozzi, Claudio
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Date Issued

2023-07-08

Publisher

Wiley-V C H Verlag Gmbh

Published in
Advanced Materials
Subjects

Chemistry, Multidisciplinary

•

Chemistry, Physical

•

Nanoscience & Nanotechnology

•

Materials Science, Multidisciplinary

•

Physics, Applied

•

Physics, Condensed Matter

•

Chemistry

•

Science & Technology - Other Topics

•

Materials Science

•

Physics

•

femtosecond laser pulses

•

magnetoelastic effect

•

multiferroic materials

•

skyrmions

•

topological materials

•

spintronics

•

room-temperature

•

dynamics

Peer reviewed

REVIEWED

Written at

EPFL

EPFL units
IPHYS-CGCP  
LQM  
Available on Infoscience
July 31, 2023
Use this identifier to reference this record
https://infoscience.epfl.ch/handle/20.500.14299/199500
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