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research article

A compact approach to higher-resolution resonant inelastic x-ray scattering detection using photoelectrons

Schunck, Jan O.
•
Buck, Jens
•
Engel, Robin Y.
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May 1, 2024
New Journal Of Physics

The detection of inelastically scattered soft x-rays with high energy resolution usually requires large grating spectrometers. Recently, photoelectron spectrometry for analysis of x-rays (PAX) has been rediscovered for modern spectroscopy experiments at synchrotron light sources. By converting scattered photons to electrons and using an electron energy analyser, the energy resolution for resonant inelastic x-ray scattering (RIXS) becomes decoupled from the x-ray spot size and instrument length. In this work, we develop PAX towards high energy resolution using a modern photoemission spectroscopy setup studying Ba2Cu3O4Cl2 at the Cu L 3-edge. We measure a momentum transfer range of 24% of the first Brillouin zone simultaneously. Our results hint at the observation of a magnon excitation below 100 meV energy transfer and show intensity variations related to the dispersion of dd-excitations. With dedicated setups, PAX can complement the best and largest RIXS instruments, while at the same time opening new opportunities to acquire RIXS at a range of momentum transfers simultaneously and combine it with angle-resolved photoemission spectroscopy in a single instrument.

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Type
research article
DOI
10.1088/1367-2630/ad4206
Web of Science ID

WOS:001218944200001

Author(s)
Schunck, Jan O.
•
Buck, Jens
•
Engel, Robin Y.
•
Kruse, Simon R.
•
Marotzke, Simon
•
Scholz, Markus
•
Mahatha, Sanjoy K.
•
Huang, Meng-Jie
•
Ronnow, Henrik M.  
•
Dakovski, Georgi
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Date Issued

2024-05-01

Publisher

Iop Publishing Ltd

Published in
New Journal Of Physics
Volume

26

Issue

5

Article Number

053008

Subjects

Physical Sciences

•

Resonant Inelastic X-Ray Scattering

•

High-Temperature Superconductor

•

Quantum Materials

•

Photoemission

•

X-Ray Spectroscopy Methods

Peer reviewed

REVIEWED

Written at

EPFL

EPFL units
LQM  
FunderGrant Number

Federal Ministry of Education and Research (BMBF)

05KS7FK2

Helmholtz Association

VH-NG-1105

Available on Infoscience
June 5, 2024
Use this identifier to reference this record
https://infoscience.epfl.ch/handle/20.500.14299/208314
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