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  4. SpiroZin1: A Reversible and pH-Insensitive, Reaction-Based, Red-Fluorescent Probe for Imaging Biological Mobile Zinc
 
research article

SpiroZin1: A Reversible and pH-Insensitive, Reaction-Based, Red-Fluorescent Probe for Imaging Biological Mobile Zinc

Rivera-Fuentes, Pablo
•
Lippard, Stephen J.
2014
ChemMedChem

A reversible, reaction-based sensor for biol. mobile zinc was designed, prepd., and characterized. The sensing mechanism of this probe is based on the zinc-induced, ring-opening reaction of spirobenzopyran to give a cyanine fluorophore that emits in the deep-red region of the electromagnetic spectrum. This probe is not activated by protons and operates efficiently in aq. soln. at pH 7 and high ionic strength. The mechanism of this reaction was studied by using a combination of kinetics expts. and DFT calcns. The biocompatibility of the probe was demonstrated in live HeLa cells.

  • Details
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Type
research article
DOI
10.1002/cmdc.201400014
Author(s)
Rivera-Fuentes, Pablo
Lippard, Stephen J.
Date Issued

2014

Published in
ChemMedChem
Volume

9

Start page

1238

End page

1243

Subjects

aqueous solution

•

article

•

benzopyran derivative

•

Benzopyrans

•

biocompatibility

•

bioinorganic chemistry

•

biosensors

•

chemical reaction kinetics

•

chemistry

•

confocal microscopy

•

coordination chemistry

•

Coordination Complexes

•

coordination compound

•

density functional theory

•

electromagnetic field

•

fluorescence imaging

•

fluorescent dye

•

Fluorescent Dyes

•

HeLa cell line

•

HeLa Cells

•

human

•

human cell

•

Humans

•

Hydrogen-Ion Concentration

•

ionic strength

•

metabolism

•

Microscopy

•

Confocal

•

pH

•

priority journal

•

proton

•

pyridine derivative

•

Pyridines

•

ring opening

•

spectrofluorometry

•

Spectrometry

•

Fluorescence

•

spirobenzopyran

•

SpiroZin1

•

synthesis

•

thermodynamics

•

Thermodynamics

•

unclassified drug

•

zinc

•

Zinc

•

zinc reversible fluorescence biosensor cell imaging

Editorial or Peer reviewed

REVIEWED

Written at

OTHER

EPFL units
LOCBP  
Available on Infoscience
October 30, 2019
Use this identifier to reference this record
https://infoscience.epfl.ch/handle/20.500.14299/162488
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