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  4. Persistence of Magnetism in Atomically Thin MnPS3 Crystals
 
research article

Persistence of Magnetism in Atomically Thin MnPS3 Crystals

Long, Gen
•
Henck, Hugo
•
Gibertini, Marco  
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April 8, 2020
Nano Letters

The magnetic state of atomically thin semiconducting layered antiferromagnets such as CrI3 and CrCI3 can be probed by forming tunnel barriers and measuring their resistance as a function of magnetic field (H) and temperature (T). This is possible because the spins within each individual layer are ferromagnet cally aligned and the tunneling magnetoresistance depends on the relative orientation of the magnetization in adjacent layers. The situation is different for systems that are antiferromagnetic within the layers in which case it is unclear whether magnetoresistance measurements can provide information about the magnetic state. Here, we address this issue by investigating tunnel transport through atomically thin crystals of MnPS3, a van der Waals semiconductor that in the bulk exhibits easy-axis antiferromagnetic order within the layers. For thick multilayers below T similar to 78 K, a T-dependent magnetoresistance sets in at mu H-0 similar to 5 T and is found to track the boundary between the antiferromagnetic and the spin-flop phases known from bulk measurements. We show that the magnetoresistance persists as thickness is reduced with nearly unchanged characteristic temperature and magnetic field scales, albeit with a different dependence on H, indicating the persistence of magnetism in the ultimate limit of individual monolayers.

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Type
research article
DOI
10.1021/acs.nanolett.9b05165
Web of Science ID

WOS:000526413400029

Author(s)
Long, Gen
Henck, Hugo
Gibertini, Marco  
Dumcenco, Dumitru
Wang, Zhe
Taniguchi, Takashi
Watanabe, Kenji
Giannini, Enrico
Morpurgo, Alberto F.
Date Issued

2020-04-08

Publisher

AMER CHEMICAL SOC

Published in
Nano Letters
Volume

20

Issue

4

Start page

2452

End page

2459

Subjects

Chemistry, Multidisciplinary

•

Chemistry, Physical

•

Nanoscience & Nanotechnology

•

Materials Science, Multidisciplinary

•

Physics, Applied

•

Physics, Condensed Matter

•

Chemistry

•

Science & Technology - Other Topics

•

Materials Science

•

Physics

•

mnps3

•

2d magnetism

•

spin flop

•

tunneling transport

•

phase-transitions

•

critical-behavior

•

2d materials

•

antiferromagnets

•

ferromagnetism

•

anisotropy

•

dynamics

Editorial or Peer reviewed

REVIEWED

Written at

EPFL

EPFL units
THEOS  
Available on Infoscience
May 2, 2020
Use this identifier to reference this record
https://infoscience.epfl.ch/handle/20.500.14299/168525
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