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  4. Electromagnon dispersion probed by inelastic X-ray scattering in LiCrO2
 
research article

Electromagnon dispersion probed by inelastic X-ray scattering in LiCrO2

Toth, Sandor
•
Wehinger, Bjorn
•
Rolfs, Katharina
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2016
Nature Communications

Inelastic X-ray scattering with meV energy resolution (IXS) is an ideal tool to measure collective excitations in solids and liquids. In non-resonant scattering condition, the cross-section is strongly dominated by lattice vibrations (phonons). However, it is possible to probe additional degrees of freedom such as magnetic fluctuations that are strongly coupled to the phonons. The IXS spectrum of the coupled system contains not only the phonon dispersion but also the so far undetected magnetic correlation function. Here we report the observation of strong magnon-phonon coupling in LiCrO2 that enables the measurement of magnetic correlations throughout the Brillouin zone via IXS. We find electromagnon excitations and electric dipole active two-magnon excitations in the magnetically ordered phase and heavily damped electromagnons in the paramagnetic phase of LiCrO2. We predict that several (frustrated) magnets with dominant direct exchange and non-collinear magnetism show surprisingly large IXS cross-section for magnons and multi-magnon processes.

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Type
research article
DOI
10.1038/ncomms13547
Web of Science ID

WOS:000388658700001

Author(s)
Toth, Sandor
•
Wehinger, Bjorn
•
Rolfs, Katharina
•
Birol, Turan
•
Stuhr, Uwe
•
Takatsu, Hiroshi
•
Kimura, Kenta
•
Kimura, Tsuyoshi
•
Rønnow, Henrik M.  
•
Ruegg, Christian
Date Issued

2016

Publisher

Nature Research

Published in
Nature Communications
Volume

7

Article Number

13547

Subjects

MPBH

URL

URL

http://lqm.epfl.ch
Editorial or Peer reviewed

REVIEWED

Written at

EPFL

EPFL units
LQM  
Available on Infoscience
January 24, 2017
Use this identifier to reference this record
https://infoscience.epfl.ch/handle/20.500.14299/133629
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