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  4. Dark-level trapping, lateral confinement, and built-in electric field contributions to the carrier dynamics in c-plane GaN/AlN quantum dots emitting in the UV range
 
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research article

Dark-level trapping, lateral confinement, and built-in electric field contributions to the carrier dynamics in c-plane GaN/AlN quantum dots emitting in the UV range

Hrytsaienko, M.
•
Gallart, M.
•
Ziegler, M.
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February 7, 2021
Journal Of Applied Physics

c-plane GaN/AlN quantum dots (QDs) are promising zero-dimensional quantum nanostructures that exhibit single photon emission properties up to room temperature and even above. In this context, it is of prime interest to gain a deeper insight into the recombination dynamics of photogenerated electron-hole pairs captured by such dots. Hence, in this work, we study the time-resolved photoluminescence (PL) properties in the low injection regime and at cryogenic temperatures of c-plane GaN/AlN QD ensembles emitting above the bulk GaN bandgap in order to properly understand the nature of the recombination channels behind the observed non-exponential decay time profiles. Such decays reveal the existence of a relaxation channel competing with the radiative recombination one. It is thus observed that for the former process the dynamics is independent of the dot height, which is attributed to a reversible nonradiative transfer that could be mediated by a spin-flip process to a dark-level state. The radiative recombination process is recognizable thanks to the characteristic dependence of its lifetime with the emission energy, which is well accounted for by the built-in electric field inherent to quantum nanostructures grown along the c axis and the variations in the lateral confinement at play in such QDs. Those conclusions are drawn from the analysis of the time evolution of the PL spectra by means of a simple analytical model that enables to exclude any screening of the built-in electric field.

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Type
research article
DOI
10.1063/5.0038733
Web of Science ID

WOS:000617500300001

Author(s)
Hrytsaienko, M.
•
Gallart, M.
•
Ziegler, M.
•
Cregut, O.
•
Tamariz, S.
•
Butte, R.  
•
Grandjean, N.  
•
Hoenerlage, B.
•
Gilliot, P.
Date Issued

2021-02-07

Publisher

AMER INST PHYSICS

Published in
Journal Of Applied Physics
Volume

129

Issue

5

Article Number

054301

Subjects

Physics, Applied

•

Physics

•

lifetime

•

excitons

•

photons

•

light

Peer reviewed

REVIEWED

Written at

EPFL

EPFL units
LASPE  
Available on Infoscience
March 26, 2021
Use this identifier to reference this record
https://infoscience.epfl.ch/handle/20.500.14299/176563
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