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  4. Flexible application of biogas upgrading membranes for hydrogen recycle in power-to-methane processes
 
research article

Flexible application of biogas upgrading membranes for hydrogen recycle in power-to-methane processes

Gantenbein, Andreas
•
Witte, Julia
•
Biollaz, Serge M. A.
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January 16, 2021
Chemical Engineering Science

Direct methanation of biogas converts the CO2 in raw-biogas to methane, enabling higher methane yield and an elelctricity storage option via Power-to-Gas. As the thermodynamic equilibrium limits the methane yield, unreacted hydrogen has to be removed and recycled to reach grid injection quality. We tested a commercial biogas upgrading membrane for hydrogen recycling at TRL 5. Based on the experi-ments, we developed a concept, which flexibly combines biogas upgrading and methanation post upgrading in a single unit. This allows switching between the two operation modes, which can improve the economic benefit of the system. The hollow fibre membrane module was tested simulating the methanation product gas (biomethane, 12% H-2 in CH4) and biogas (40% CO2 in CH4) in pressure ranges of 3-9 bar. In both cases, grid injection limitations (<2% H-2, <4% CO2) were reached at pressures of 6-8 bar. (c) 2020 Elsevier Ltd. All rights reserved.

  • Details
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Type
research article
DOI
10.1016/j.ces.2020.116012
Web of Science ID

WOS:000584396400008

Author(s)
Gantenbein, Andreas
Witte, Julia
Biollaz, Serge M. A.
Krocher, Oliver  
Schildhauer, Tilman Jy
Date Issued

2021-01-16

Publisher

PERGAMON-ELSEVIER SCIENCE LTD

Published in
Chemical Engineering Science
Volume

229

Article Number

116012

Subjects

Engineering, Chemical

•

Engineering

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power-to-gas

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biogas

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membrane

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upgrading

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flexibility

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direct catalytic methanation

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gas separation

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model

Editorial or Peer reviewed

REVIEWED

Written at

EPFL

EPFL units
GR-KRO  
Available on Infoscience
June 19, 2021
Use this identifier to reference this record
https://infoscience.epfl.ch/handle/20.500.14299/179012
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