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  4. Imaging Nonradiative Point Defects Buried in Quantum Wells Using Cathodoluminescence
 
research article

Imaging Nonradiative Point Defects Buried in Quantum Wells Using Cathodoluminescence

Weatherley, Thomas F. K.  
•
Liu, Wei  
•
Osokin, Vitaly
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June 23, 2021
Nano Letters

Crystallographic point defects (PDs) can dramatically decrease the efficiency of optoelectronic semiconductor devices, many of which are based on quantum well (QW) heterostructures. However, spatially resolving individual nonradiative PDs buried in such QWs has so far not been demonstrated. Here, using high-resolution cathodoluminescence (CL) and a specific sample design, we spatially resolve, image, and analyze nonradiative PDs in InGaN/GaN QWs at the nanoscale. We identify two different types of PDs by their contrastin behavior with temperature and measure their densities from 10(14) cm(-3) to as high as 10(16) cm(-3). Our CL images clearly illustrate the interplay between PDs and carrier dynamics in the well: increasing PD concentration severely limits carrier diffusion lengths, while a higher carrier density suppresses the nonradiative behavior of PDs. The results in this study are readily interpreted directly from CL images and represent a significant advancement in nanoscale PD analysis.

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Type
research article
DOI
10.1021/acs.nanolett.1c01295
Web of Science ID

WOS:000668003400042

Author(s)
Weatherley, Thomas F. K.  
•
Liu, Wei  
•
Osokin, Vitaly
•
Alexander, Duncan T. L.  
•
Taylor, Robert A.
•
Carlin, Jean-Francois  
•
Butte, Raphael  
•
Grandjean, Nicolas  
Date Issued

2021-06-23

Publisher

AMER CHEMICAL SOC

Published in
Nano Letters
Volume

21

Issue

12

Start page

5217

End page

5224

Subjects

Chemistry, Multidisciplinary

•

Chemistry, Physical

•

Nanoscience & Nanotechnology

•

Materials Science, Multidisciplinary

•

Physics, Applied

•

Physics, Condensed Matter

•

Chemistry

•

Science & Technology - Other Topics

•

Materials Science

•

Physics

•

semiconductor

•

point defects

•

quantum wells

•

cathodoluminescence

•

ingan

•

imaging

•

radiative lifetime

•

recombination

•

dependence

•

emission

•

gaas

Editorial or Peer reviewed

REVIEWED

Written at

EPFL

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Available on Infoscience
July 17, 2021
Use this identifier to reference this record
https://infoscience.epfl.ch/handle/20.500.14299/179967
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