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review article

Recent advances in interfacial engineering for high-efficiency perovskite photovoltaics

Wang, Zhijie
•
Gong, Cheng
•
Zhang, Cong
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June 1, 2025
DeCarbon

Through strategies such as process optimization, solvent selection, and component tuning, the crystallization of perovskite materials has been effectively controlled, enabling perovskite solar cells (PSCs) to achieve over 25 ​% power conversion efficiency (PCE). However, as PCE continues to improve, interfacial issues within the devices have emerged as critical bottlenecks, hindering further performance enhancements. Recently, interfacial engineering has driven transformative progress, pushing PCEs to nearly 27 ​%. Building upon these developments, this review first summarizes the pivotal role of interfacial modifications in elevating device performance and then, as a starting point, provides a comprehensive overview of recent advancements in normal, inverted, and tandem structure devices. Finally, based on the current progress of PSCs, preliminary perspectives on future directions are presented.

  • Details
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Type
review article
DOI
10.1016/j.decarb.2025.100107
Scopus ID

2-s2.0-86000757535

Author(s)
Wang, Zhijie

Fudan University

Gong, Cheng

Jiangxi University of Science and Technology

Zhang, Cong

Henan Polytechnic University

Zhao, Chenxu  

École Polytechnique Fédérale de Lausanne

Su, Tzu Sen

National Taiwan University of Science and Technology

Li, Haiyun

Fudan University

Zhang, Hong

Fudan University

Date Issued

2025-06-01

Published in
DeCarbon
Volume

8

Article Number

100107

Subjects

Defect passivation

•

Device stability

•

Energy level alignment

•

Interfacial engineering

•

Ion migration

•

Perovskite solar cells

Editorial or Peer reviewed

REVIEWED

Written at

EPFL

EPFL units
LCOM  
FunderFunding(s)Grant NumberGrant URL

Education Ministry of China

Doctoral Foundation of Henan Polytech-nic University

B2024-72

National Natural Science Foundation of China

52302229,62404072

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Available on Infoscience
March 25, 2025
Use this identifier to reference this record
https://infoscience.epfl.ch/handle/20.500.14299/248219
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