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research article

In-Plane Magnetic Anisotropy of Fe Atoms on Bi2Se3(111)

Honolka, J.
•
Khajetoorians, A. A.
•
Sessi, V.
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2012
Physical Review Letters

The robustness of the gapless topological surface state hosted by a 3D topological insulator against perturbations of magnetic origin has been the focus of recent investigations. We present a comprehensive study of the magnetic properties of Fe impurities on the prototypical 3D topological insulator Bi2Se3 using local low-temperature scanning tunneling spectroscopy and integral x-ray magnetic circular dichroism techniques. Single Fe adatoms on the Bi2Se3 surface, in the coverage range approximate to 1% of a monolayer, are heavily relaxed into the surface and exhibit a magnetic easy axis within the surface plane, contrary to what was assumed in recent investigations on the supposed opening of a gap. Using ab initio approaches, we demonstrate that an in-plane easy axis arises from the combination of the crystal field and dynamic hybridization effects.

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Type
research article
DOI
10.1103/PhysRevLett.108.256811
Web of Science ID

WOS:000305569200004

Author(s)
Honolka, J.
Khajetoorians, A. A.
Sessi, V.
Wehling, T. O.
Stepanow, S.
Mi, J. -L.
Iversen, B. B.
Schlenk, T.
Wiebe, J.
Brookes, N. B.
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Date Issued

2012

Published in
Physical Review Letters
Volume

108

Article Number

256811

Subjects

Augmented-Wave Method

•

Ultrasoft Pseudopotentials

•

Topological Insulators

•

Surface

Editorial or Peer reviewed

REVIEWED

Written at

EPFL

EPFL units
LSEN  
Available on Infoscience
July 20, 2012
Use this identifier to reference this record
https://infoscience.epfl.ch/handle/20.500.14299/84017
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