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research article

Advancing non-equilibrium ARPES experiments by a 9.3 eV coherent ultrafast photon source

Cilento, F.
•
Crepaldi, A.  
•
Manzoni, G.
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2016
Journal Of Electron Spectroscopy And Related Phenomena

The quest for investigating the non-equilibrium dynamics of the band structure of strongly-correlated materials over their entire Brillouin zone is a primary objective. However, the actual ultrafast UV light sources are not suitable for addressing several critical questions in the field. Here we report on a novel light source generating sub-250 fs, 9.3 eV photon energy light pulses at 250 kHz repetition rate, obtained via third-harmonic generation in Xe of frequency-doubled 50 fs laser pulses at 1.55 eV. By reporting the measured band dispersion of a Cu(111) crystal and the non-equilibrium dynamics of the Bi2Se3 topological insulator, we prove that this source is suitable for studying the non-equilibrium dynamics of the entire Fermi surface of several complex materials, with high signal statistics and limited space-charge effect. (C) 2015 Elsevier B.V. All rights reserved.

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Type
research article
DOI
10.1016/j.elspec.2015.12.002
Web of Science ID

WOS:000371940400002

Author(s)
Cilento, F.
Crepaldi, A.  
Manzoni, G.
Sterzi, A.
Zacchigna, M.
Bugnon, Ph.
Berger, H.  
Parmigiani, F.
Date Issued

2016

Publisher

Elsevier Science Bv

Published in
Journal Of Electron Spectroscopy And Related Phenomena
Volume

207

Start page

7

End page

13

Editorial or Peer reviewed

REVIEWED

Written at

EPFL

EPFL units
LSE  
Available on Infoscience
April 1, 2016
Use this identifier to reference this record
https://infoscience.epfl.ch/handle/20.500.14299/125366
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